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Description: Raw experimental data for the publication "External Acidity as Performance Descriptor in Polyolefin Cracking using Zeolite-Based Materials". Contains: Large dataset of ramped and isothermal TGA for zeolite catalyzed cracking of polypropylene (over 300 experiments), activity data for cracking of dimethylpentane, semi-batch cracking, and zeolite characterization using Ar physisorption, Hg-porosimetry, Py-IR and TTBP-IR. Check the GitHub repository (https://github.com/MyonicS/External_Acidity_Paper) for additional details and code processing the underlying data.